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This dataset collection contains Chemical Ablation Model version 3 (CABMOD3) simulations of metal ablation from meteoroids and Meteoric Ablation Simulator (MASI) sodium and nickel ablation experimental data. This experiment was undertaken as part of Natural Environment Research Council (NERC) First study of the global Nickel and Aluminium Layers in the upper atmosphere (NIALL) project (NE/P001815/1). This project aimed to make the first ever study of Ni and Al chemistry in the mesosphere/lower thermosphere.